Association for Research at University Nuclear Accelerators - Interconnected collective of 11 institutions
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Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview 1
ARUNA in a Nutshell Nuclear Science Advisory Committee (NSAC) Long Range Plan 2015 “We recommend increasing investment in small-scale and mid-scale projects and initiatives that enable forefront LECM 2021 – ARUNA Overview research at universities and laboratories. […]” ARUNA’s core mission Maximize and optimize the use of all nuclear accelerator facilities at universities in the U.S. ARUNA institutions host world-unique experimental capabilities/facilities, including high-intensity photon beams, ultra-low background conditions, intense neutron sources, high-intensity stable and radioactive ion beams. Provide unique training opportunities for the next-generation nuclear workforce 20% of US nuclear-physics PhDs come from ARUNA institutions Mount innovative science programs and complement science program of National Laboratories ARUNA institutions perform research in nuclear structure, nuclear astrophysics, to test fundamental symmetries, and to apply nuclear-physics techniques to national security, nuclear power and to benefit society. 2 ARUNA members are main contributors to the science program at FRIB, ANL and other national laboratories.
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview 3
Graduates from ARUNA institutions (2019-2021) ARUNA graduates went on to work at, e.g., FRIB, the different national laboratories including ANL, BNL, LLNL, and PNNL, at NASA, at the US Department of Defense, at Northrop Grumman, Duo Security, and Intel Corp. 2019 2020 2021 LECM 2021 – ARUNA Overview Abromeit, Brittany (Ph.D., Tabor, FSU) Aguilar, Sebastian (M.S., Ahn, Notre Dame) Agarwal, Shiva (M.S., Famiano, WMU) Anastasiou, Maria (Ph.D., Wiedenhöver, FSU) Anderson, Tyler (Ph.D., Collon, Notre Dame) Asher, Benjamin (Ph.D., Almaraz-Calderon, FSU) Bagdasarova, Yelena (Ph.D., Garcia, UW) Bennett, Eames (Ph.D., Christian, TAMU) Gerken, Nathan (Ph.D., Almaraz-Calderon, FSU) Bartram, Chelsea (Ph.D., Henning, UNC) Caves, Louis (M.S., Bardayan, Notre Dame) Karrick, Hayden (M.S., Famiano, WMU) Chyzh, Roman (Ph.D., Tribble, TAMU) Dowen, Lori (Ph.D., Iliadis, UNC) Liu, Peifan (Ph.D., Wu, Duke) Cooper, Andrew (Ph.D., Champagne, UNC) Glennon, Kevin (Ph.D., Folden, TAMU) McGuinness, Sean (Ph.D., Peaslee, Notre Dame) Dermigny, Jack (Ph.D., Iliadis, UNC) Howard, Kevin (Ph.D., Garg, Notre Dame) Perello, Jesus (Ph.D., Almaraz-Calderon, FSU) Drees, Eric (Ph.D., Young, NCSU) Huestis, Patricia (Ph.D., Couder/LaVerne, Notre Dame) Sensharma, Nirupama (Ph.D., Wiescher, Notre Dame) Du, Xiaojian (Ph.D., Rapp, TAMU) Jedele, Andrea (Ph.D., Yenello, TAMU) Siegel, Mark (M.S., Famiano, WMU) Friesen, Forrest (Ph.D., Howell, Duke) Li, Xiaqing (Ph.D., Gao, Duke) Soltesz, Doug (Ph.D., Meisel, Ohio U.) Gilardy, Gwenaelle (Ph.D., Couder, Notre Dame) Little, David (Ph.D., Janssens, UNC) Vande Kolk, Bryant (Ph.D., Wiescher, Notre Dame) Gillis, Tom (Ph.D., Wilkerson, UNC) Liu, Qian (Ph.D., Wiescher, Notre Dame) Whitehead, Taylor (Ph.D., Holt, TAMU) Giri, Rekam (Ph.D., Brune, Ohio U.) Long, Jacob (Ph.D., Brodeur, Notre Dame) Hall, Matthew (Ph.D., Bardayan, Notre Dame) Malone, Ronald (Ph.D., Howell, Duke) Heacock, Benjamin (Ph.D., Huffman & Young, NCSU) Marshall, Caleb (Ph.D., Longland, NCSU) Hooker, Josh (Ph.D., Rogachev, TAMU) Paneru, Som (Ph.D., Brune, Ohio U.) Hunt, Sean (Ph.D., Iliadis, UNC) Reingold, Craig (Ph.D., Simon, Notre Dame) Jayatissa, Heshani (Ph.D., Rogachev, TAMU) Rubino, Elizabeth (Ph.D., Tabor, FSU) Kelly, James (Ph.D., Brodeur, Notre Dame) Siegl, Kevin (Ph.D., Aprahamian, Notre Dame) Koehler, Katrina Elizabeth (Ph.D., Famiano, WMU) Skulski, Michael (Ph.D., Collon, Notre Dame) Lubna, Rebeka (Ph.D., Tabor, FSU) Strauss, Sabrina (Ph.D., Aprahamian, Notre Dame) Meijer, Samuel (Ph.D., Wilkerson, UNC) Upadhyayula, Sriteja (Ph.D., Rogachev, TAMU) Raeger, Jamin (Ph.D., Hennig, UNC) Xiong, Weizhi (Ph.D., Gao, Duke) Sultana, Irin (M.S., Meisel, Ohio U.) Villafana, Kalisa (Ph.D., Riley, FSU) Viola, Merinda (Ph.D., Folden, TAMU) Yang, Zhidong (Ph.D., Fries, TAMU) Yingying, Chen (Ph.D., Wiescher, Notre Dame) 4
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview 5
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions Precise measurements of 6He and LECM 2021 – ARUNA Overview 19Ne beta spectra via Cyclotron Radiation Emission Spectroscopy → Searching for chirality-flipping interactions 6
CENPA at U. of Washington University of Washington Precise measurements of 6He and 19Ne beta spectra via Cyclotron Radiation Emission Spectroscopy (CRES) LECM 2021 – ARUNA Overview → Searching for chirality-flipping interactions (tensor currents to shine path beyond Standard Model) Collaboration with ANL, Mainz, NCSU, PNNL, Texas A&M, Tulane → Measure beta energy by frequency of cyclotron radiation: = 2 / Multi-track electron event 7 spectrum
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Detailed studies of the Hoyle state with TexAT TPC, neutron detection and 211At production 8
Experiment performed at Cyclotron Institute using MARS beamline, 12N beam implantation Measurement of direct decay of 12C in Hoyle state Stringent limits on the Efimov state in 12C Direct-looking event Additional Efimov state exceeds triple-alpha rate at 6 x 107 K required for red giant phase β-feeding strength
Experiment performed at Cyclotron Institute using MARS beamline, 12N beam implantation Measurement of direct decay of 12C in Hoyle state Stringent limits on the Efimov state in 12C Direct-looking event Additional Efimov state exceeds triple-alpha rate at 6 x 107 K required for red giant phase β-feeding strength
Experiment performed at Cyclotron Institute using MARS beamline, 12N beam implantation Measurement of direct decay of 12C in Hoyle state Stringent limits on the Efimov state in 12C Direct-looking event Additional Efimov state exceeds triple-alpha rate at 6 x 107 K required for red giant phase β-feeding strength
Clear n/γ PSD and separation TexNeut - p-terphenyl neutron detector array between n’s in different crystals. n’s 6 individual 2 x 2 x 2 cm3 p-terphenyl crystals in ‘pseudobar’ geometry. Readout PMT at either end LECM 2021 – ARUNA Overview γ’s >300 keVee • Can be coupled to TexAT TPC or run in stand-alone mode • PSD-threshold 150 keVee • Position resolution (to single crystal) 300 keVee • Timing resolution < 700 ps • Commissioning expt: 9Li(p,n) – structure of 10Li(g.s) via IAS in 10Be with 48 bar array • Many exciting experiments to D.P. Scriven et al. NIMA 1010, 165492 (2021) 12 come!
At-211 Production at Texas A&M Chilled Production Water Flow Rapid recovery of At-211 by 209Bi(α,2n)211At at 28.8 MeV, 4-8 µA extraction chromatography LECM 2021 – ARUNA Overview 28.8 MeV α Dissolution of Target 6–12 M HNO3 (nitric acid) New purification method results in larger At-211 yields faster than previous methods. Purification based on newly discovered chemical interaction Experimental Chemistry of At-211 with ketones. Separations and Fundamental Background: Targeted Alpha Therapy Potential to be a curative treatment for patients after primary cancer treatment 211At is the only α-decaying isotope fulfilling the Radiolabeling for Targeted Alpha criteria for nuclear medicine applications Therapy → T1/2 > 1h → No serial decay (which could contribute 13 J.D. Burns, et al., Chem. Commun., 56, 9004-9007, 2020. J.D. Burns, et al., J. Sep. Pur., 256, 117794, 2021. to toxicity in vivo from daughters), one alpha
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Sub-barrier fusion studies, secondary γ rays for Nuclear Astrophysics, and 13C(α,n)16O for neutron background in precision neutrino experiments 14
15 LECM 2021 – ARUNA Overview NSF grant No. PHY-2011890
16 LECM 2021 – ARUNA Overview NSF grant No. PHY-2011890
17 LECM 2021 – ARUNA Overview NSF grant No. PHY-2011890
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Education, determination of water contamination and interdisciplinary work 18
Research Experience for Undergraduate Students Nitrogen Beams with a National Electrostatics Corporation Alphatross Source and LECM 2021 – ARUNA Overview a 5SDH Accelerator B. Harlow, P. A. DeYoung, and V. A. Bunnell Undergraduate Research in Physics With a careful calibration of the analyzing magnet based on 14 beams of many energies, the formation of NH- and NH2- by the ion source was confirmed. Activities at Hope College: Application: RBS characterization of thin targets (most recently with R. deSouza, Indiana University) Application/Society: Development of an inexpensive anti-Compton suppression shield to lower the minimum level of detection in proton induced γ-ray emission (PIGE) measurements. [Fluorine detection in samples to monitor water contamination in western Michigan.] Interdisciplinary Work: Biologists use the accelerator to irradiate mice to determine the effects of chronic low 19 dose radiation similar to that experienced by astronauts.
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Atomic Physics and Material Sciences using the WMU accelerator 20
LECM 2021 – ARUNA Overview Atomic Physics: Radiative Double Electron Capture for F on Graphene Clear difference! Students working inside the tank. Nefiodov AV et al 2005 Phys. Lett. A346, 158 La Mantia D S et al 2020 Phys. Rev. Lett. 124, 133401 La Mantia D S et al 2020 Phys. Rev. A. 102, 060801(R) X-Ray Spectra 21 Experimental Setup NSF PHY-1707467
LECM 2021 – ARUNA Overview Materials Science: Localized Surface Plasmon Resonance (LSPR) of metal nanoparticle (MNP) due to Ion-implanted Silver Nanoparticles for Metal-Enhanced Fluorescence coherent oscillations of conduction band electrons with incident electromagnetic Enhancement due to 4x105 No Nps radiations of a specific wavelength. LSPR is Ag Nanoparticles! 0.8 x 1016 p/cm2 1.1 x 1016 p/cm2 generated in MNP at a size smaller than the 1.3 x 1016 p/cm2 wavelength of light Fl Intensity 3x105 1.5 x 1016 p/cm2 3 x 1016 p/cm2 2x105 1x105 0 450 500 550 600 650 Wavelength (nm) Ph.D. Dissertation Emission spectra of C515 dye on bare and silver- Plasmonic field enhancement due to Singh, Manpreet, et al. Sensors 17.2 (2017): 428. Implanted quartz for different Ag ion fluences. An plasmonic coupling or hot spots for the Iqbal, Shahid, et al. AIP Advances 8.9 (2018): increase in the fluorescence intensity of C515 spherical NPs with diameter of the 5.6 nm: 095217. indicating the influence of MEF in the presence of Left: Monomer, Right: Dimer. 22 Ag implanted substrates. Metal Enhanced Fluorescence (MEF) has promising applications in the field of optical displays, bio-sensing and photodynamic therapy.
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Detailed γ-ray spectroscopy experiments after INS for constraining nuclear structure input for neutrinoless double-beta decay and scattering of fast neutrons on materials relevant for reactor design. 23
University of Kentucky Accelerator Laboratory Probing nuclear structure with fast neutrons: Neutrinoless double-beta decay and shape coexistence in Ge nuclei LECM 2021 – ARUNA Overview (n,n′γ) DSAM lifetimes τ = 28(2) fs Mixing ratios Branching ratios 74Ge Identify and characterize ẟ = +5.84+48 UKAL all low-energy −60 states Transition probabilities Arrow widths proportional to B(E2)s Transition probabilities for: Constraining 0νββ nuclear matrix PRC 95, 014327 (2017) and more coming soon! element calculations (e.g., Ge nuclei) 24 Identifying shape coexistence www.pa.uky.edu/accelerator
University of Kentucky Accelerator Laboratory Probing nuclei with fast neutrons: cross section measurements for basic science and applications LECM 2021 – ARUNA Overview 12C Angular distributions of neutron elastic and inelastic scattering cross natC Neutron (n,n) Cross Sections sections to guide R-matrix global evaluations of scattering from carbon. Important for use as a neutron standard and for reactor materials. 112,114 Cd (n,γ) cross sections important for many applications. 7Li Potential -ray production standard; large discrepancies currently exist in the neutron inelastic cross sections; best current resonance parameters are inconsistent with our understanding of 8Li nuclear structure. 19F Coolant component for molten salt reactors and passive interrogation. Difficult target because of the 90 ns isomeric first excited state. Measurements were abandoned in the 1960s because of this. Installation of new digital DAQ at UKAL should provide new opportunities to measure these cross sections. E.A. Chouinard, 24Mg Potential coolant component for molten salt reactors and used as a S.E. Evans, strengthener in aluminum alloys. Angular distributions are needed for U. Dallas verifying reaction model calculations. students, Summer 2021 Collaboration: UK, USNA, UDallas, and MS State 25 WORKFORCE DEVELOPMENT A hands-on student-run facility
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Detailed nuclear structure studies with the SE-SPS, CLARION-2 and neutron-γ coincidences to study the nucleosynthesis of galactic 26Al 26
γ-ray spectroscopy at FSU and CLARION-2 Florida State University CLARION-2 (16 active S. Ajayi Compton-supressed CLOVER detectors) is being installed at FSU. LECM 2021 – ARUNA Overview Detailed study of high- Collaboration with: spin states in 59Co E. Rubino approaching the 2nd island First experiments will of inversion. start soon! → 2019 experiment with 6 [V. Tripathi, S. Tabor, J.M. Allmond] CLARION-2 Clovers! Particle spectroscopy at the Super-Enge Split-Pole Spectrograph and Fox Lab REU program SE-SPS has been the most used device at the Fox Lab. Several high-resolution experiments ran using (d,p), (p,p’), (d,d’), (α,d) to study single-particle states, the N = 32 subshell closure (52Ca), fully-aligned states and collective structures. REU program at SE-SPS successfully continued in its 2nd year with students from Ursinus (L. Riley) and Davidson College (A. Kutchera). REU@FSU FSU REU 2021 G. McCann C. Benetti J.M. Nebel-Crosson 27 [50Ti(d,p): L. Riley, J.M. Nebel-Crosson, et al., Phys. Rev. C 103, 064309 (2021)]; [27Al(α,d)29Si: C. Benetti, S. Tabor] NSF grant No. PHY-2012522
Coincident neutron and γ-ray spectroscopy of 26Si Florida State University J. Perello Single-particle structure of the PDR in 48,50Ti LECM 2021 – ARUNA Overview 47Ti(d,p)48Ti = 1− @ HIγS Sp @SE-SPS* A. Conley resonances Sn 24Mg(3He,nγ)26Si to inform 25Al(p,γ)26Si relevant B. Kelly for nucleosynthesis of galactic 26Al. First tests for particle-γ experiments @ SE-SPS 49Ti(d,p)50Ti = 1− @ HIγS @SE-SPS* Sn Four 2×2 inches CeBr3; digital Onset of PDR beyond N = 28? CAEN DAQ → Larger array planned. Identification of PDR doorway states for direct neutron New 8-inch diameter Al scattering capture. Is the complete PDR important for (n,γ)? chamber constructed at FSU. 28 → Increases FEP efficiency by a NSF grant No. PHY-2012522 factor of 8. *targets provided by the Center for Accelerator Target Science, ANL
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Nuclear Astrophysics studies with neutrons and detailed benchmarking of simulations. 29
Ohio University (Edwards Accelerator Laboratory) Evaporation Spectra for 59Cu(p,γ) in X-ray Bursts LECM 2021 – ARUNA Overview Performed at the Edwards Accelerator Laboratory using the beam-swinger and neutron time-of-flight tunnel. The 58Ni(3He,n) double-differential cross section was used to determine the nuclear level density of 60Zn, which is the compound nucleus of the important rp-process reaction 59Cu(p,γ). We Doug Soltesz (Ph.D., 2021) found that at X-ray burst temperatures, the level density has an unexpected plateau and is on the border of validity for the statistical regime. 3He+4He Scattering for Solar 3He(α,γ) Performed at TRIUMF using the (Scattering of Nuclei in Inverse Kinematics) SONIK chamber Determined s-wave scattering length for 3He+4He, which helped constrain the 3He(α,γ) astrophysical S-factor. This S- factor is the main uncertainty in predictions of the solar neutrino flux from 7Be and 8B. This uncertainty hinders benchmarks of solar models. 30 Som Paneru (Ph.D., 2020)
Ohio University (Edwards Accelerator Laboratory) 13C(α,n) Cross Section for Geoneutrino Detector Backgrounds Benchmarking MCNP for … Everything! and s-Process Nucleosynthesis LECM 2021 – ARUNA Overview [Voinov+ PRC 2020] Cross section measured for [Brandenburg+, in prep.] d(n,2n) @ En = 15 MeV Aimed at improving diagnostics for inertial confinement fusion facilities, such as NIF and Kristyn Brandenburg OMEGA. Found that JENDL describes the data better than the ENDF Measured excitation function of 13C(α,n) at energies of interest for neutrino-detector backgrounds, where existing data was known to library that is used in MCNP*. *Monte-Carlo N-Particle Transport Code have a significant systematic uncertainty. Bayesian R-Matrix Analyses of t(d,n) for Big-Bang Nucleosynthesis & Internal Confinement Fusion Daniel Odell Implemented Bayesian methods in R-matrix data analysis, using t(d,n) as a proof of (postdoc) principle. Currently being expanded to other light-ion [Odell+ arXiv:2105.06541] reactions of interest for nuclear astrophysics. 31
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Fission fragment studies, new opportunities at HIγS, studies at LENA and upgrade, the TUNL SPS Nuclear Astrophysics program. 32
RApid Clover+CeBr3 array at HIγS Belt-driven LECM 2021 – ARUNA Overview Irradiated Target Transfer System Fission Product Yields (FPYs) measured in collaboration with LLNL and LANL Measured > 60 fission products with t1/2 > 0.5 s from 8 (16) Clover-type HPGe* and 12 (2x2 inches) 235U, 238U, 239Pu CeBr3 detectors Energy dependent FPY data at En = 0.57, 2.0, 4.6, 9.0, Higher rates in HPGe possible due to segmentation Higher granularity 14.8 MeV CeBr3 detectors have no intrinsic activity WIENER Mpod high-voltage control system Molly DeLuca @ RABITTS Automatic LN2 filling system (ANL) TUNL REU student, summer 2021 Optional replacement of HPGe with LaBr3 available at HIγS *Provided by the Clovershare Consortium, the US Naval Academy, the US army research lab, and TUNL. 33
Jack Dermigny, PhD 2019; Dermigny et al., PRC 102, 014609 (2020) Study of 30Si(p,γ) to understand abundance anomalies in globular clusters Caleb Marshall, First observation of resonance and precise PhD 2020 LECM 2021 – ARUNA Overview measurement of another Marshall et al., PRC Reduce recommended reaction rate by a factor of 10 23Na(3He,d)24Mg to constrain Na Significant reduction in uncertainty production in globular clusters Influence of previously LENA γγ-coincidence spectrometer unobserved resonance (surrogate for 23Na(p,γ)24Mg) Discovered new energy for key 133-keV resonance Previous rate Factor of two increase in recommended reaction rate New rate On 435-keV resonance; HPGe spectrum 34 γ-ray energy [keV]
Jack Dermigny, PhD 2019; Dermigny et al., PRC 102, 014609 (2020) Study of 30Si(p,γ) to understand abundance anomalies in globular clusters Caleb Marshall, First observation of resonance and precise PhD 2020 LECM 2021 – ARUNA Overview measurement of another Marshall et al., PRC Reduce recommended reaction rate by a factor of 10 23Na(3He,d)24Mg to constrain Na Significant reduction in uncertainty production in globular clusters Influence of previously LENA γγ-coincidence spectrometer unobserved resonance (surrogate for 23Na(p,γ)24Mg) Discovered new energy for key 133-keV resonance Previous rate Factor of two increase in recommended reaction rate New rate On 435-keV resonance; HPGe spectrum 35 γ-ray energy [keV]
Jack Dermigny, PhD 2019; Dermigny et al., PRC 102, 014609 (2020) Study of 30Si(p,γ) to understand abundance anomalies in globular clusters Caleb Marshall, First observation of resonance and precise PhD 2020 LECM 2021 – ARUNA Overview measurement of another Marshall et al., PRC Reduce recommended reaction rate by a factor of 10 23Na(3He,d)24Mg to constrain Na Significant reduction in uncertainty production in globular clusters Influence of previously LENA γγ-coincidence spectrometer unobserved resonance (surrogate for 23Na(p,γ)24Mg) Discovered new energy for key 133-keV resonance Previous rate Factor of two increase in recommended reaction rate New rate On 435-keV resonance; HPGe spectrum 36 γ-ray energy [keV]
Jack Dermigny, PhD 2019; Dermigny et al., PRC 102, 014609 (2020) Study of 30Si(p,γ) to understand abundance anomalies in globular clusters Caleb Marshall, First observation of resonance and precise PhD 2020 LECM 2021 – ARUNA Overview measurement of another Marshall et al., PRC Reduce recommended reaction rate by a factor of 10 23Na(3He,d)24Mg to constrain Na Significant reduction in uncertainty production in globular clusters Influence of previously LENA γγ-coincidence spectrometer unobserved resonance (surrogate for 23Na(p,γ)24Mg) Discovered new energy for key 133-keV resonance Previous rate Factor of two increase in recommended reaction rate New rate On 435-keV resonance; HPGe spectrum 37 γ-ray energy [keV]
Jack Dermigny, PhD 2019; Dermigny et al., PRC 102, 014609 (2020) Study of 30Si(p,γ) to understand abundance anomalies in globular clusters Caleb Marshall, First observation of resonance and precise PhD 2020 LECM 2021 – ARUNA Overview measurement of another Marshall et al., PRC Reduce recommended reaction rate by a factor of 10 23Na(3He,d)24Mg to constrain Na Significant reduction in uncertainty production in globular clusters Influence of previously LENA γγ-coincidence spectrometer unobserved resonance (surrogate for 23Na(p,γ)24Mg) Discovered new energy for key 133-keV resonance Previous rate Factor of two increase in recommended reaction rate New rate On 435-keV resonance; HPGe spectrum 38 γ-ray energy [keV]
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview Study of environmental pollution with low-energy ion beams. 39
Ion-Beam Analysis of Environmental Pollution Lead Contamination in Soil Around Bridges LECM 2021 – ARUNA Overview PFAS Contamination From Fire-Fighting Foam 1.0MV Tandem Peaslee+ Environmental Science & Technology Letters (2020) Source: United States Environmental Protection Agency (EPA) Per- and polyfluoroalkyl substances (PFAS) are a group of man-made chemicals that have been in use since the 1940s, and are (or have been) found in many consumer products like cookware, 40 food packaging, and stain repellants.
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions See upcoming talk by A. Rogers LECM 2021 – ARUNA Overview 41
Recent Research Highlights UMass Lowell Radiation Lab Main Facilities: 5.5-MV Van de Graaff 1-MW Research Reactor LECM 2021 – ARUNA Overview 6 graduate students, ~6-8 undergrads, 1-2 postdocs Analysis of BNL BLIP isotopes • Medical isotopes produced at BNL BLIP are brought to UML for Large Volume HPGe detailed assay. Implanted targets and • The Lowell array of Compton- suppressed HPGe detectors are characterization used for precise measurements of • Lifetime measurements of excited states yield, dose and impurities using well-characterized implanted Beam targets. Compton-suppressed HPGe Array • Deuteron beams (~2 A) are energy degraded and implanted in a target foil. Exit window • Elastic Recoil Detection Analysis (ERDA) using 4He beams to characterize the External-beam development depth and number of implanted 2H. • Ion-beam analysis and high- • Future project: Develop low-energy ion throughput irradiations of in-air source for ion-implantation applications. samples. 42 • Initial test using PIGE for identifying and quantifying 19F from PFAS.
Recent Research Highlights UMass Lowell Radiation Lab Main Facilities: 5.5-MV Van de Graaff 1-MW Research Reactor LECM 2021 – ARUNA Overview 6 graduate students, ~6-8 undergrads, 1-2 postdocs Analysis of BNL BLIP isotopes • Medical isotopes produced at BNL BLIP are brought to UML for Large Volume HPGe detailed assay. Implanted targets and • The Lowell array of Compton- suppressed HPGe detectors are characterization used for precise measurements of • Lifetime measurements of excited states yield, dose and impurities using well-characterized implanted Beam targets. Compton-suppressed HPGe Array • Deuteron beams (~2 A) are energy degraded and implanted in a target foil. Exit window • Elastic Recoil Detection Analysis (ERDA) using 4He beams to characterize the External-beam development depth and number of implanted 2H. • Ion-beam analysis and high- • Future project: Develop low-energy ion throughput irradiations of in-air source for ion-implantation applications. samples. 43 • Initial test using PIGE for identifying and quantifying 19F from PFAS.
An Outreach Example: Inspiring the next generation 2021 in-person camp LECM 2021 – ARUNA Overview 2020 online camp 2020 online camp 2020 online camp 44
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions LECM 2021 – ARUNA Overview 45
Association for Research at University Nuclear Accelerators Interconnected collective of 11 institutions Thank you for your attention. LECM 2021 – ARUNA Overview 46
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