Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI

 
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Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI
atmosphere
Communication
Can We Vacuum Our Air Pollution Problem Using
Smog Towers?
Sarath Guttikunda *          and Puja Jawahar
 Urban Emissions, New Delhi 110019, India; puja@urbanemissions.info
 * Correspondence: sguttikunda@urbanemissions.info
                                                                                                      
 Received: 29 July 2020; Accepted: 28 August 2020; Published: 29 August 2020                          

 Abstract: In November 2019, the Supreme Court of India issued a notification to all the states in the
 National Capital Region of Delhi to install smog towers for clean air and allocated INR 36 crores
 (~USD 5.2 million) for a pilot. Can we vacuum our air pollution problem using smog towers?
 The short answer is “no”. Atmospheric science defines the air pollution problem as (a) a dynamic
 situation where the air is moving at various speeds with no boundaries and (b) a complex mixture
 of chemical compounds constantly forming and transforming into other compounds. With no
 boundaries, it is unscientific to assume that one can trap air, clean it, and release into the same
 atmosphere simultaneously. In this paper, we outline the basics of atmospheric science to describe
 why the idea of vacuuming outdoor air pollution is unrealistic, and the long view on air quality
 management in Indian cities.

 Keywords: India; Delhi; air quality; controls; smog towers; filtration systems

1. Introduction
      Air pollution is a major health risk worldwide—outdoor PM2.5 (particulate matter) and
Ozone pollution accounted for an estimated 3 million and 0.5 million premature deaths,
respectively, and household (indoor) air pollution for an additional 1.6 million premature deaths [1].
Corresponding numbers for India are 680,000 for outdoor PM2.5 , 145,000 for outdoor ozone, and 480,000
for household pollution. Similar estimates were presented by researchers and scientists from the Indian
institutes [2–6]. In all the studies, the very young and the old are particularly vulnerable.
      The year 2020 is an aberration in the pollution trends, with the COVID-19 lockdowns and a range
of restrictions for all the sectors [7]. Across India, ambient air pollution levels improved as much as 50%
compared to the annual trends for the same period in the previous year [8]. A summary of the data
from all the cities with at least one continuous air monitoring station is included in the Supplementary
Materials. Following the pandemic, epidemiological work on COVID-19 patients suggests that the risk
of mortality is higher among the population exposed to chronic PM2.5 and NO2 pollution [9,10].
      One key lesson from the COVID-19 lockdowns worldwide, is that air pollution can be reduced
locally and globally by reducing the emissions at the sources. This was witnessed in the data from
the ground-based monitors worldwide and satellite retrievals over India, China, Italy, and the United
States [11–13]. The measures enacted during the lockdowns are unprecedented, but the results are
evidence that we eventually need to control the emissions at the sources for “clean air”.
      While the messages are clear that high air pollution is the leading cause of health impacts and
“clean air” is only possible by addressing the emissions at the sources, in November 2019, the Supreme
Court of India issued a notification to all the states in the National Capital Region of Delhi (NCR) to
install smog towers. These giant filtering systems are being pursued as a control mechanism only in the
absence of real action to control the emissions at the sources and the continuing incidence of high air
pollution levels in Delhi and other major cities. Examples discussed in the notification for replication

Atmosphere 2020, 11, 922; doi:10.3390/atmos11090922                            www.mdpi.com/journal/atmosphere
Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI
While the messages are clear that high air pollution is the leading cause of health impacts and
“clean air” is only possible by addressing the emissions at the sources, in November 2019, the
Supreme Court of India issued a notification to all the states in the National Capital Region of Delhi
(NCR) to install smog towers. These giant filtering systems are being pursued as a control mechanism
only in the
Atmosphere   absence
           2020, 11, 922 of real action to control the emissions at the sources and the continuing incidence
                                                                                                       2 of 11
of high air pollution levels in Delhi and other major cities. Examples discussed in the notification for
replication are (a) a 100 m high purification tower in Xi’an, China [14] and (b) experimental large
are (a) a 100 m high purification tower in Xi’an, China [14] and (b) experimental large vacuum cleaners
vacuum cleaners called Wind Augmentation and Air Purifying Units (WAYU) were deployed in the
called Wind Augmentation and Air Purifying Units (WAYU) were deployed in the cities of Delhi,
cities of Delhi, Mumbai, and Bengaluru, with no operational details, and (c) a smaller version of the
Mumbai, and Bengaluru, with no operational details, and (c) a smaller version of the Xi’an smog tower
Xi’an smog tower in Delhi (Figure 1). The latter designs also include “mist makers” to initiate
in Delhi (Figure 1). The latter designs also include “mist makers” to initiate coagulation and induce wet
coagulation and induce wet scavenging of the particles. The units installed in Delhi and Mumbai
scavenging of the particles. The units installed in Delhi and Mumbai were designed by the National
were designed by the National Environmental Engineering Research Institute (NEERI) and Indian
Environmental Engineering Research Institute (NEERI) and Indian Institute of Technology (Mumbai)
Institute of Technology (Mumbai) and inaugurated by the then Minister of Environment [15].
and inaugurated by the then Minister of Environment [15].

                      (a)                                            (b)                                     (c)

      Figure 1. Examples of ambient filtering systems: (a) a smog tower from Xi’an, China, (Image edited
      Figure 1. Examples of ambient filtering systems: (a) a smog tower from Xi’an, China, (Image edited
      from South China Morning Post), (b) a Wind Augmentation and Air Purifying Unit (WAYU) in Delhi,
      from South China Morning Post), (b) a Wind Augmentation and Air Purifying Unit (WAYU) in Delhi,
      and (c) a smaller version of Xi’an’s filtering system in Delhi.
      and (c) a smaller version of Xi’an’s filtering system in Delhi.
      A fundamental question remains, “can we vacuum our air pollution problem using smog towers
      A fundamental
and mist    makers”? question
                           The shortremains,
                                        answer“can       we vacuum
                                                   is “no”.   The idea ourofair  pollutionwhat
                                                                              removing      problem      using smog
                                                                                                    is already   in thetowers
                                                                                                                          air is
and   mist  makers”?      The   short   answer     is “no”.  The   idea  of   removing     what
unrealistic, given the dynamic nature of air pollution, which moves and transforms simultaneously. is  already   in  the  air is
unrealistic,   given   the  dynamic     nature   of  air pollution,  which     moves   and  transforms
In this paper, we outline the basics of atmospheric science to describe why the idea of vacuuming            simultaneously.
In this paper,
outdoor            we outline
           air pollution         the basics of
                             is unscientific,   andatmospheric
                                                      the long viewscience   to describe
                                                                        on air             why the ideainofIndian
                                                                                 quality management               vacuuming
                                                                                                                          cities.
outdoor    air  pollution   is unscientific,   and   the long  view   on air  quality  management
In India, PM2.5 is considered the main criteria pollutant for environmental compliance and public         in  Indian  cities.  In
India,  PM  2.5 is considered the main criteria pollutant for environmental compliance and public health,
health, and all of the discussion in this paper is about PM.
and all of the discussion in this paper is about PM.
2. The Sciences
2. The Sciences
      The definition of atmospheric science can be explained via the three basic sciences—Mathematics,
      Theand
Physics,     definition
                 Chemistry. of atmospheric science can be explained via the three basic sciences—
Mathematics, Physics, and Chemistry.
2.1. Mathematics
2.1. Mathematics
      Mathematics relates to the “quantification” of the problem. In a box model version of a city
      Mathematics
(Figure  2), the size relates    to the
                        of the city   and“quantification”
                                           the height of theofinversion
                                                                   the problem.layer In  a determine
                                                                                      will box modelthe     version
                                                                                                                amountof aofcity
                                                                                                                             air
(Figure 2),
present       the size
          at any    givenofinstance.
                             the city and
                                        Thethe   height of
                                             inversion       the is
                                                          layer   inversion    layerlayer
                                                                    an invisible      will of
                                                                                           determine
                                                                                               air, which  thedetermines
                                                                                                                amount ofthe  air
present
total     at any
      volume     of given   instance.
                    air available   for The  inversion
                                        horizontal    andlayer   is an
                                                           vertical     invisible
                                                                     mixing.    Thislayer  of isair,
                                                                                      height         which determines
                                                                                                  determined     by prevalentthe
total volume
surface            of air air
         temperature,      available    for horizontal
                               temperature     at the groundandandvertical
                                                                      uppermixing.      This height
                                                                               layers, humidity           is determined
                                                                                                     levels,   and land cover,by
prevalent
all varyingsurface
              in timetemperature,
                        and space. Thereair temperature
                                              is seasonalityatassociated
                                                               the groundwith  andtheupper  layers,layer—highest
                                                                                       inversion       humidity levels,     and
                                                                                                                        during
landsummer
the   cover, all    varying
                months    andinlowest
                                 time and    space.
                                        during         There is
                                                  the winter     seasonality
                                                              months.    This is associated   with the
                                                                                   a typical trend         inversion
                                                                                                      for most   of thelayer—
                                                                                                                        inland
cities in India [16]. The coastal cities like Chennai and Mumbai experience lesser variation across the
seasons due to the constant presence of land–sea breeze.
Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI
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 highest during the summer months and lowest during the winter months. This is a typical trend for
 most of the inland cities in India [16]. The coastal cities like Chennai and Mumbai experience lesser
Atmosphere
 variation2020, 11, 922
           across    the seasons due to the constant presence of land–sea breeze.               3 of 11

                                (a)                                                                   (b)

      Figure 2. Depiction of a box model pollution calculation with varying inversion heights (a) for summer
       Figure 2. Depiction of a box model pollution calculation with varying inversion heights (a) for
      months and (b) for winter months.
       summer months and (b) for winter months.
      Pollution (in the units of µg/m3 ) is defined as mass over volume, where mass is the emission load
       Pollution
and volume           (in amount
                 is the   the unitsofof airμg/m
                                                  3) is defined as mass over volume, where mass is the emission
                                             present.    In the summer months, a higher volume of air means more
 load and
room         volume
        for lateral   andis the   amount
                             vertical        of airand
                                        mixing,      present.   In thefor
                                                          vice versa     summer       months,
                                                                             the winter          a higher
                                                                                           months.          volume
                                                                                                       For the   sameofamount
                                                                                                                            air meansof
emissions in all the months, concentrations are bound to be higher in the winter months andamount
 more   room    for  lateral   and   vertical  mixing,     and  vice  versa    for the  winter   months.    For  the   same     lower
 ofthe
in  emissions
         summer   in months.
                      all the months,      concentrations
                                   For “clean    air” and lowerare bound      to be higherthe
                                                                      concentrations,         in requirement
                                                                                                  the winter months        andhigher
                                                                                                                   is either     lower
 in the   summer      months.      For   “clean   air”  and   lower    concentrations,       the
inversion layer height or lower emissions. It is next to impossible to alter meteorology; however,requirement       is either   higher
 inversionemissions
reducing      layer height       or lower
                            should            emissions.
                                      be relatively    easy.It is next to impossible to alter meteorology; however,
 reducing
      In theemissions
               box model,    should    be relatively
                                 we assumed        thateasy.
                                                          emissions remain constant over months. This is not true.
Emissions
       In the box model, we assumed that case
              are   also   seasonal,    which    in  the         of India
                                                           emissions        are higher
                                                                        remain             in the
                                                                                    constant   over winter   months
                                                                                                       months.    This from
                                                                                                                         is notspace
                                                                                                                                  true.
heating
 Emissions needs
               are [17]
                     alsoalong      withwhich
                            seasonal,      a lowering
                                                  in the in   mixing
                                                           case         height,
                                                                 of India           furtherincompounding
                                                                              are higher       the winter months the airfrompollution
                                                                                                                                 space
problem.     A hypothetical
 heating needs       [17] along case withisa illustrated
                                              lowering ininmixing
                                                                Table 1height,
                                                                           for what     couldcompounding
                                                                                     further    be the changes    theinair
                                                                                                                         thepollution
                                                                                                                               overall
pollution   when     the   city  size  expands,    emissions     halve   or   double,   or for  changes
 problem. A hypothetical case is illustrated in Table 1 for what could be the changes in the overall       in the   meteorological
conditions.
 pollution when All the
                      thecalculations       assumeemissions
                            city size expands,        a steady state
                                                                  halvecondition.
                                                                          or double,The       worst-case
                                                                                         or for  changes in scenario    is when the
                                                                                                               the meteorological
emissions    double     and   the   mixing   height   drops    to a quarter     of the  norm,
 conditions. All the calculations assume a steady state condition. The worst-case scenario is  resulting    in a  700%    increase
                                                                                                                             when thein
the  overall double
 emissions     pollution.andDuring
                                the mixingthe winter
                                               height haze
                                                         dropsepisodes,
                                                                 to a quarter areasof between
                                                                                      the norm,Punjab,      Haryana,
                                                                                                    resulting  in a 700%   and  Delhi
                                                                                                                              increase
experience     these   conditions      [18,19]—emissions        nearly    double     compared      to
 in the overall pollution. During the winter haze episodes, areas between Punjab, Haryana, and Delhi  summer     months      with   the
addition    of  agricultural     residue    burning     and  the  onset   of   winter   season
 experience these conditions [18,19]—emissions nearly double compared to summer months with the   requiring   more     biomass     and
coal combustion
 addition             to support
            of agricultural          space burning
                                  residue    heating, with     a simultaneous
                                                         and the   onset of winter   dropseason
                                                                                          in the surface
                                                                                                   requiringandmore
                                                                                                                  air temperatures.
                                                                                                                        biomass and
Typical
 coal combustion to support space heating, with a simultaneous drop in the surface mand
           day-time     mixing     layer   heights   are  1000–2000     m   in  the  summer     months    and   100–200         in the
                                                                                                                                     air
winter    months.     Typical    night-time    heights     are half  of this.
 temperatures. Typical day-time mixing layer heights are 1000–2000 m in the summer months and
100–200 m in the winter months. Typical night-time heights are half of this.
      Table 1. A hypothetical pollution calculation for a city using a steady state box model method.
      W = width of the city; L = length of the city; H = mixing height; E = emissions.
       Table 1. A hypothetical pollution calculation for a city using a steady state box model method. W =
       width of Study
                the city;
                       andL =Institution
                              length of the city; H = mixing
                                                         W height;
                                                                 L E = emissions.
                                                                          H       E      Pollution %Change
                    Study
                  Base case, and
                             all asInstitution
                                    usual                       1.0       W
                                                                          1.0     L 1.0 H          1.0E     Pollution
                                                                                                               1.0      %Change
                                                                                                                         0%
    City size doubles in width and length and no
                  Base                                          2.0       2.0 1.0 1.0 1.0 1.0                 0.25        −75%
               change  in case, all as usual
                          the emissions                                   1.0              1.0                 1.0          0%
    Emission doubles,
     City size doubleseverything
                         in widthelse
                                   andis length
                                         the same   1.0
                                                and no                     1.0         1.0         2.0         2.0       +100%
                                                                          2.0    2.0         1.0    1.0       0.25         −75%
                 change
      Mixing height      in the
                    doubles,    emissions
                             everything else is
                                                                1.0        1.0         2.0         1.0         0.5        −50%
                     the same
      Emission doubles, everything else is the same                       1.0    1.0         1.0    2.0        2.0         +100%
       Mixing height halves, everything else is
                                                                1.0        1.0         0.5         1.0         2.0       +100%
                      the same
  Mixing height doubles, everything else is the same                      1.0    1.0         2.0    1.0        0.5         −50%
     Emission doubles and mixing height halves                  1.0        1.0         0.5         2.0         4.0       +300%
   Mixing height
     Emission    halves,
              doubles andeverything elseisis the same
                          mixing height                                   1.0    1.0         0.5    1.0        2.0         +100%
                                                                1.0        1.0       0.25          2.0         8.0       +700%
                        one quarter
        Emission halves and everything else is
                                                                1.0        1.0         1.0         0.5         0.5        −50%
                      the same
Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI
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     Mathematically, for a given set of seasonal patterns in meteorology, especially over the
Indo-Gangetic plain, the best option is to cut the emissions at the sources and disperse the emissions to
 Atmosphere 2020, 11, x FOR PEER REVIEW                                                             5 of 13
farther distances via better urban planning.
 2.2. Physics
2.2. Physics
       Physics relates to the “movement” of the problem. A popular saying is that “pollution knows no
      Physics relates to the “movement” of the problem. A popular saying is that “pollution knows
 boundaries”. The box model assuming closed walls in Figure 2 and Table 1 is good to illustrate the
no boundaries”. The box model assuming closed walls in Figure 2 and Table 1 is good to illustrate
 point that emissions are key for any increase and decrease in pollution levels. Simultaneously,
the point that emissions are key for any increase and decrease in pollution levels. Simultaneously,
 meteorology plays an important role in determining how much of those emissions stay in the box,
meteorology plays an important role in determining how much of those emissions stay in the box,
 determined by the horizontal wind components (U and V), or how much of those emissions will stay
determined by the horizontal wind components (U and V), or how much of those emissions will stay
 close to the surface, determined by the vertical wind component (W) (Figure 3).
close to the surface, determined by the vertical wind component (W) (Figure 3).

                               Figure 3. Three-dimensional motion of air through a city.
                               Figure 3. Three-dimensional motion of air through a city.
       This adds two new dimensions to the air pollution problem: (a) the air is not static over the
       This adds two new dimensions to the air pollution problem: (a) the air is not static over the city—
city—between wind speeds of 1 m/s and 2 m/s, the latter is pushing twice the amount of air through the
 between wind speeds of 1 m/s and 2 m/s, the latter is pushing twice the amount of air through the
city boundaries; (b) the air from outside the boundary carries outside emissions, which add to the total
 city boundaries; (b) the air from outside the boundary carries outside emissions, which add to the
emissions inside the city. Similarly, emissions from inside the city will be carried to a city downwind.
 total emissions inside the city. Similarly, emissions from inside the city will be carried to a city
This is called “long-range transport” of pollution—sometimes this is an exchange of pollution between
 downwind. This is called “long-range transport” of pollution—sometimes this is an exchange of
the cities and sometimes between the states. For example, a city like Delhi is surrounded by satellite
 pollution between the cities and sometimes between the states. For example, a city like Delhi is
cities Gurugram (from the state of Haryana) in the West and Noida (from the state of Uttar Pradesh)
 surrounded by satellite cities Gurugram (from the state of Haryana) in the West and Noida (from the
in the East. There is constant movement of vehicles between these cities and in a map of urban
 state of Uttar Pradesh) in the East. There is constant movement of vehicles between these cities and
built-up area, it is difficult to draw a closed box [20]. In this case, depending on the wind direction,
 in a map of urban built-up area, it is difficult to draw a closed box [20]. In this case, depending on the
emissions from each of these cities are affecting the others downwind.
 wind direction, emissions from each of these cities are affecting the others downwind.
       The effect of long-range transport is also prominent during the seasonal dust storms (May–June)
originating    from
       The effect   ofthe   Middle transport
                        long-range     East or the is Thar   desert in the
                                                      also prominent           statethe
                                                                           during      of seasonal
                                                                                          Rajasthan    [21],
                                                                                                     dust    and agricultural
                                                                                                          storms    (May–June)
residue   burning
 originating    from(April–May
                        the Middleand     October–November)
                                        East or the Thar desertoriginating
                                                                        in the statemostly     from the[21],
                                                                                        of Rajasthan     states of agricultural
                                                                                                              and   Punjab and
Haryana
 residue burning (April–May and October–November) originating mostly from the states emissions
           [22].   In  both  cases,  seasonal   wind    speeds    are  high  enough     to pick   up  and push   the  of Punjab
into
 and the   higher[22].
       Haryana       altitudes,
                          In bothsupport     inter-state
                                     cases, seasonal         transport,
                                                          wind    speeds and      affectenough
                                                                            are high      the pollution
                                                                                                    to picklevels
                                                                                                             up and downwind.
                                                                                                                       push the
The   overall into
 emissions    known   thehorizontal    advectionsupport
                           higher altitudes,        and vertical    mixingtransport,
                                                              inter-state     schemes are   andmore  complex
                                                                                                  affect       than described
                                                                                                         the pollution    levels
in  this paper.
 downwind. The overall known horizontal advection and vertical mixing schemes are more complex
 thanGuttikunda
        described in  etthis
                         al. (2019)
                              paper.[16] presents an analysis for 20 Indian cities, documenting contributions of
emissions inside and outside the city airsheds. On average, 30% of the pollution observed in these cities
       Guttikunda
originates   outsideetthe al. city
                              (2019)   [16] presents
                                   limits.  For citiesan in analysis
                                                            North India for 20  Indian
                                                                             like        cities, Amritsar,
                                                                                   Ludhiana,     documenting andcontributions
                                                                                                                  Chandigarh,
 of  emissions   inside   and    outside  the  city  airsheds.    On   average,
the long-range transport contribution is more than 50% on an annual basis.         30%   of the  pollution   observed   in these
 citiesThe
         originates     outside    the  city  limits.   For   cities   in  North    India    like
            movement of the pollution also includes scavenging—dry deposition when the pollutants  Ludhiana,    Amritsar,   and
 Chandigarh,      the  long-range     transport   contribution      is  more   than   50%   on
are in contact with a surface and wet deposition during the rains. The dry deposition rates for an  annual   basis.
variousThepollutants
            movement     areofdetermined
                                the pollutionby also
                                                 the surface
                                                       includes  roughness,
                                                                   scavenging—drysoil moisture    content,
                                                                                           deposition       andthe
                                                                                                         when     wind  speeds.
                                                                                                                     pollutants
are in contact with a surface and wet deposition during the rains. The dry deposition rates for various
pollutants are determined by the surface roughness, soil moisture content, and wind speeds. Under
windy conditions and over dry surfaces, we have lesser deposition of the particulates, and vice versa
on the trees with enough moisture on the leaves.
Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI
Atmosphere 2020, 11, 922                                                                                                       5 of 11

Under windy conditions and over dry surfaces, we have lesser deposition of the particulates, and vice
Atmosphere 2020, 11, x FOR PEER REVIEW                                                         6 of 13
versa on the trees with enough moisture on the leaves.
2.3. Chemistry
 2.3. Chemistry
       Chemistry relates to the “composition” of the problem—the critical one of the three sciences, as
        Chemistry relates to the “composition” of the problem—the critical one of the three sciences,
it links PM2.5, PM10, SO2, NO2, CO and ozone directly to all known health impacts. Of the six
 as it links PM2.5 , PM10 , SO2 , NO2 , CO and ozone directly to all known health impacts. Of the six
pollutants, the most critical is PM2.5, and its chemical composition is different in space and time
pollutants, the most critical is PM2.5 , and its chemical composition is different in space and time [23,24].
[23,24]. While the first five pollutants are part of direct emissions, ozone is a secondary compound
While the first five pollutants are part of direct emissions, ozone is a secondary compound formed in
formed in the atmosphere in the presence of NOx and hydrocarbons.
 the atmosphere in the presence of NOx and hydrocarbons.
       AA sample
           sampleof   ofPMPM2.52.5can
                                    canprovide
                                         provide     information
                                                   information       not
                                                                   not   only
                                                                       only  ononhowhowmuchmuch    pollution
                                                                                                pollution       there
                                                                                                            there        is, but
                                                                                                                    is, but   alsoalso
                                                                                                                                   on
 on  the  fuel    origins  of   the   mass   on   the  filter. Figure  4 presents    a summary
the fuel origins of the mass on the filter. Figure 4 presents a summary of the key marker metals,    of the  key  marker       metals,
 elements, and
elements,      and compounds
                      compounds associated
                                        associated with with major
                                                               major sources.
                                                                      sources. There
                                                                                 There areare overlaps
                                                                                               overlaps between
                                                                                                           between the  the sources
                                                                                                                              sources
 and   the  ratio   of the markers       also vary     significantly,  which   allows   for statistically
and the ratio of the markers also vary significantly, which allows for statistically apportioning source    apportioning       source
 contributions.      These   markers       range    from    metals  from  direct  combustion      of
contributions. These markers range from metals from direct combustion of fuels, like coal and diesel,fuels,  like coal    and   diesel,
 to contributions
to   contributionsfrom   fromother     gases,
                                   other        likelike
                                           gases,     SO2 SOforming   sulphate
                                                               2 forming         aerosols
                                                                            sulphate        (in a series
                                                                                         aerosols    (in aofseries
                                                                                                              reactions
                                                                                                                      of involving
                                                                                                                           reactions
 ozone    and     some   intermediate        radicals),
involving ozone and some intermediate radicals),            NO  x forming    nitrate  aerosols    and   hydrocarbons
                                                                       NOx forming nitrate aerosols and hydrocarbons         forming
 secondary
forming          organic aerosols
            secondary                   (via 500+
                           organic aerosols           known
                                                    (via        reactions
                                                         500+ known        with ozone
                                                                        reactions   withandozoneintermediate     radicals)
                                                                                                   and intermediate            [25,26].
                                                                                                                            radicals)
 Ozone     is a   by-product       of these  500+     reactions.   Most  of  the  chemical    transformation
[25,26]. Ozone is a by-product of these 500+ reactions. Most of the chemical transformation between                between      gases
 and   aerosols     takes  place      during   the   long-range     transport—in      other   words,
gases and aerosols takes place during the long-range transport—in other words, a significant portion    a significant     portion   of
 thethe
of    PM PM2.52.5samples
                   samplescollected
                             collectedininthe  thecity
                                                     cityare
                                                           arethere
                                                                therebecause
                                                                       because ofof the
                                                                                     the emissions
                                                                                          emissions originating         outside the
                                                                                                        originating outside        the
 city [16].   The   secondary       nature  of  the   PM      originating  from   sources   not  likely  within
city [16]. The secondary nature of the PM2.52.5originating from sources not likely within a city boundary,        a city   boundary,
 complicates the
complicates        the overall
                       overall pollution
                                   pollution control
                                               control strategy.
                                                           strategy.

                    Figure
                    Figure 4.
                           4. Key
                              Key metal
                                  metal and
                                        and ion
                                            ion markers
                                                markers of
                                                        of various
                                                           various sources
                                                                   sources contributing to PM
                                                                           contributing to PM2.5
                                                                                              2.5. .

3. Do
3. DoSmog
      SmogTowers
          Towers Work?
                 Work?
      For managing
      For managingoutdoor
                        outdoorairairpollution,
                                      pollution,thetheanswer
                                                         answeris is  still
                                                                  still     “no”.
                                                                         “no”.      Atmospheric
                                                                                 Atmospheric         science
                                                                                                 science      defines
                                                                                                          defines   the the
                                                                                                                        air
 air pollution  problem    as (a) a dynamic   situation     where    the  air  is moving    at
pollution problem as (a) a dynamic situation where the air is moving at various speeds with no various   speeds   with   no
 boundaries, and
boundaries,    and (b)
                   (b) aacomplex
                          complex mixture
                                     mixture of
                                             of chemical
                                                 chemical compounds
                                                              compounds constantly
                                                                               constantly forming
                                                                                            forming andand transforming
                                                                                                            transforming
 into other compounds.      With   no boundaries,     it is unscientific    to assume    that
into other compounds. With no boundaries, it is unscientific to assume that one can trap air,  one  can trap  air,clean
                                                                                                                   cleanit,
                                                                                                                          it,
 and release
and   release into
               into the same atmosphere simultaneously. Expecting       Expecting filtering
                                                                                      filtering units
                                                                                                  units to
                                                                                                         to provide
                                                                                                             provide any
                                                                                                                       any
 noticeable results
noticeable   results at
                     at the
                         the community
                             community level
                                           level is
                                                  is unrealistic.
                                                     unrealistic. This
                                                                     This isis illustrated
                                                                               illustrated in
                                                                                            in a back-of-the-envelope
                                                                                                  back-of-the-envelope
 calculation for
calculation   for Delhi
                  Delhi (Table
                          (Table 2)
                                  2) using two pilots under consideration,
                                                                   consideration, (a)  (a) T1: aa smog
                                                                                                   smog tower
                                                                                                          tower inin Xi’an
                                                                                                                     Xi’an
(China) designed to filter 10 million m3 of air every day; (b) T2: a smaller version of T1 piloted in
Delhi’s Lajpat number market in January 2020, with a capacity of 600,000 m3/day.

    For these calculations, we considered Delhi’s airshed, including its satellite cities Gurugram,
Noida, Greater Noida, Ghaziabad, Faridabad, and Rohtak, covering an area of 7000 sq.km (~84 km ×
Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI
Atmosphere 2020, 11, 922                                                                                                                                         6 of 11

(China) designed to filter 10 million m3 of air every day; (b) T2: a smaller version of T1 piloted in
Delhi’s Lajpat number market in January 2020, with a capacity of 600,000 m3 /day.

                Table 2. Outdoor air pollution filtering efficiency of the smog towers in Delhi’s airshed.

                   Variable                               Delhi’s Airshed                 T1: Xi’an Smog Tower                      T2: Delhi’s 2020 Pilot
      Filtering capacity under full
                                                                                                        400,000                                  25,000
         implementation (m3 /h)
    Average airshed volume (m3 /h),                  1,209,600 million in the
     calculated using inputs from                    summer 120,960 million
                Table 3                                   in the winter
                                                                                          0.000033% in the summer                  0.000002% in the summer
   Filtering efficiency as the amount
                                                                                             and 0.00033% in the                      and 0.00002% in the
        of air filtered in one hour
                                                                                                   winter                                   winter
                                                                                            3,024,000 units in the                  50,000,000 units in the
     Number of towers required at
                                                                                            summer and 302,400                      summer and 5,000,000
            full capacity
                                                                                             units in the winter                      units in the winter
                                                     The Supreme Court of
                                                                                                                                      INR 700,000 (~USD
                                                     India allocated INR 36               Unknown; reported pilot
                   Unit cost                                                                                                       10,000) + operations and
                                                    crores (~USD 5.2 million)              cost is USD 10 million
                                                                                                                                         maintenance
                                                       for replication of T1
      Required capital cost for full
                                                                                             USD 15,725 billion                         USD 500 billion
       implementation in Delhi
         Required operations and
         maintenance costs for full                                                                     HIGH                                     HIGH
         implementation in Delhi

      Table 3. Summary of all day (AD), daytime (DT), and nighttime (NT) averages (± standard deviations)
      of mixing heights (MH in m), near surface temperature (T in ◦ C), and near surface wind speeds (WS in
      m/s) by month. Data is extracted from Weather Research Forecasting (WRF) model simulations using
      the National Centers for Environmental Prediction (NCEP) reanalysis fields for the year 2018.
 Variable   January      February      March         April        May          June          July         August      September     October      November December
 MH–AD      298 ± 58     516 ± 94     926 ± 198    1075 ± 254   1243 ± 307   1054 ± 244    573 ± 240     505 ± 152    462 ± 123     501 ± 91      350 ± 73     286 ± 71
 MH–DT      557 ± 118    974 ± 187    1801 ± 393   2066 ± 501   2377 ± 640   1855 ± 485    994 ± 450     906 ± 269    827 ± 239     959 ± 184     651 ± 129    534 ± 140
 MH–NT       39 ± 8       57 ± 56      51 ± 18      84 ± 45      109 ± 60    254 ± 124     153 ± 85      104 ± 58     97 ± 105       43 ± 13       50 ± 33      38 ± 8
  T–DT      18.9 ± 1.8   24.2 ± 2.8   30.5 ± 2.6   35.5 ± 2.4   39.4 ± 2.7   39.0 ± 3.2    33.9 ± 2.9    33.0 ± 2.1   31.4 ± 2.2    30.0 ± 1.6    25.3 ± 1.5   18.8 ± 2.2
  T–NT      9.9 ± 1.5    15.3 ± 2.5   19.6 ± 1.8   26.3 ± 2.2   31.1 ± 1.8   34.0 ± 2.3    30.6 ± 2.1    29.3 ± 1.3   26.5 ± 1.1    21.8 ± 1.8    17.5 ± 1.9   11.1 ± 2.8
 WS–AD      2.7 ± 0.7    2.8 ± 0.9     3.1 ± 0.6    3.8 ± 0.8    3.7 ± 0.9    4.5 ± 1.2    3.1 ± 0.7     2.7 ± 0.7    2.8 ± 0.9     2.5 ± 0.5     2.7 ± 0.7    2.4 ± 0.6

      For these calculations, we considered Delhi’s airshed, including its satellite cities Gurugram, Noida,
Greater Noida, Ghaziabad, Faridabad, and Rohtak, covering an area of 7000 sq.km (~84 km × 84 km).
Table 3 presents a summary of mixing heights, near surface temperature, and wind speeds for the
year 2018. The average wind speed in the domain is 4 m/s (=14.4 km/h) in the summer months and
2 m/s (=7.2 km/h) in the winter months. Similarly, the average mixing heights are 1000 m and 200 m,
respectively. This translates to an average exchange of 1,209,600 million m3 /h and 120,960 million
m3 /h of air in the summer and winter months, respectively (city side * speed * mixing height)—this
calculation assumes a steady state with constant flow of air and no vertical mixing.
      The concept of vacuum cleaning has worked in closed environments. For example, (a) in a closed
room, if the doors and windows remain shut, then an air purifier is an efficient way to clean the
air [27]. This emulates a box model containing a constant amount of air with limited movement.
When purifying the closed room, all the dust is collected on a filter, which requires either cleaning or
replacement after some time, and a clean disposal of the dust collected. During high pollution days,
the frequency of cleaning and replacement is more (b) at the end of a combustion unit, with flue gas
moving at a constant flow rate in one direction, like a power plant boiler with a chimney. The system
will include an inlet for polluted air and an outlet for cleaned air. This system is designed to trap
Can We Vacuum Our Air Pollution Problem Using Smog Towers? - MDPI
Atmosphere 2020, 11, 922                                                                               7 of 11

emissions at the source, before entering the atmosphere at the top of the chimney. In this case, all the
dust (fly ash) from the cyclone bags or electrostatic precipitators or filters also need clean collection and
disposal [28]. (c) In a subway tunnel, where the air flow is limited and prone to increased exposure
levels, a purifier will induce an artificial air flow, diluting the incoming air, and thus reducing the
overall exposure levels. None of these examples present the use of filtering systems to clean the
air permanently.
     In an outdoor environment, at best these systems are a demonstration of a filtering system with
negligible efficiencies (Table 2), whose performance at a power plant, or at any of the end of the pipe
applications where the emissions originate, is the most efficient.

4. Taking a Long View on Air Quality Management
     The air pollution problem in India is year-round [29,30]. The winter months (November,
December, January, and February) are the worst, with stagnant meteorology stifling the lateral and
vertical movement of pollution, low temperatures pushing the need for space heating, which is
mostly met using biomass [17], and some seasonal emissions from agricultural residue burning [22].
These are in addition to the all-year combustion of petrol, diesel, gas, coal, and waste in the transport,
industrial, and domestic sectors, and resuspended from the construction activities and traffic on the
roads. The monsoon months (June, July, and August) are the best, with enhanced wet scavenging
across the country.
     The air pollution problem in India is not limited to the cities. An analysis of annual average
PM2.5 concentrations, using a combination of satellite retrievals and global emission inventories for the
period of 1998–2018, suggests that 60% of the districts do not meet the national ambient standard of
40 µg/m3 and 98% do not meet the WHO guideline of 10 µg/m3 [31]. Typically, North Indian districts
are more adversely affected from chronic air pollution.
     The judicial system played a central role in several air pollution decisions in India:
•    In 1998, the Supreme Court ruled to convert public transport buses and para-transit vehicles to
     run on compressed natural gas (CNG). This was a public interest litigation, which also led to
     other emission control measures in Delhi [32,33]. CNG conversion was the most successful for
     the transport sector and, in the early 2000s, the city of Delhi witnessed a reduction in emissions
     and pollution. However, the scale of replacement has not been replicated in any other Indian city
     since, and the overall bus fleet composition in Delhi has remained the same irrespective of the
     growing demand [34].
•    In 2015, three toddlers filed a public interest ligation in the Supreme Court of India, to request
     a full ban on the sale of fireworks. In an apparent victory for cleaner air, in November 2016,
     the Court ordered a complete ban on the sale of firecrackers in the NCR. What seemed to be a
     progressive measure was, however, annulled by a ‘temporary’ ruling, when the ban was lifted
     with the caveat that the ban will be reinstituted if there is evidence that fireworks are a major
     pollutant during the festive season.
•    In 2018, the Supreme Court ruled in favour of the introduction of BS-VI standard vehicles
     nationwide, starting 1 April 2020, instead of the original plan for 2025 under the auto fuel policy.
•    In 2019, the Supreme Court ruled in favour of an immediate ban on the use of pet coke (with high
     sulphur content) in all industries in the NCR by June 2019.
     Time and again, judicial interventions have resulted in putting pressure on the respective agencies
to implement long-term measures for long-term benefits.
     Non-judicial interventions proposed and implemented for improving air quality and health are:
•    In 2015, the Government of India launched the smart cities program for 100 cities. While air
     quality was not explicitly mentioned as the environment indicator, the proposed activities were
     designed to benefit overall air quality. These included a ranking system to evaluate the waste
     management programs, road cleaning, and street greening in the cities.
Atmosphere 2020, 11, 922                                                                          8 of 11

•    In December 2016, Delhi proposed the Graded Responsibility Action Plan (GRAP), a series
     of measures to enforce under poor, very poor, severe and emergency levels of pollution [35].
     These decisions are made based on a 48-h running average of the air quality index, calculated using
     hourly PM2.5 and PM10 levels. This plan is now an example for other cities in the Indo-Gangetic
     Plain to replicate. A missing link in the program is an independent body with teeth to clamp
     down on offending polluters across states.
•    The Ministry of Petroleum and Natural Gas took an important first step with the Pradhan Mantri
     Ujjwala Yojana (PMUY) in 2016, providing liquified petroleum gas (LPG) connections to the
     poorest households. As of September 2019, the PMUY has connected 80 million beneficiaries by
     directly transferring subsidies to the bank accounts of women in these households and improving
     indoor and outdoor health [36]. While the number of connections is on the rise, there are barriers
     to LPG uptake, which need to be addressed [37].
•    In April 2015, a parliamentary standing committee proposed new emission standards for all the
     coal-fired thermal power plants. These standards were ratified in December 2015, tightening the
     standards for PM and introducing standards for SO2 , NOx , and mercury for the first time.
     If implemented in full, these standards are expected to yield a 50% drop in the PM2.5 (primary
     and secondary) pollution from these plants [38,39]. All the power plants are expected to comply
     in 2022.
•    Financial support from the Government of India for the Faster Adoption and Manufacturing
     of Electric Vehicles (FAME) program, made electric vehicles (EVs) a new policy and economic
     choice for small- and large-scale applications. The program now includes subsides for two-,
     three-, and four-wheelers and the introduction of EV buses into the public transportation system.
     The Delhi transport corporation is expected to receive its first 1000 buses in 2021–2022 and the
     Delhi government is promoting EVs to account for 25% of new registrations by 2024.
      In 2019, the Ministry of Environment, Forest and Climate Change (MoEFCC) announced the
National Clean Air Programme (NCAP) for 122 non-attainment cities from 20 states and three union
territories [40]. Under the NCAP, every city is required to prepare a list of actions necessary to
reduce their PM2.5 levels by 20–30%, compared to 2017, by 2024. The authors of [41] present a review
of these action plans, summarizing the key action points that all the cities want to implement as:
(a) augmenting public transport, (b) eradicating road and construction dust, (c) abolishing open waste
burning, (d) promoting clean cooking, (e) implementing industrial emission standards, (f) increasing
ambient monitoring capacity, and (g) raising public awareness. While improving ambient monitoring
capacity and raising public awareness are short-term activities (with long-term maintenance), all others
are part of long-term planning, designed to reduce emissions at the sources.
      Following the approval of the 102 NCAP city action plans by MoEFCC, the prevalence of
pollution episodes in October–November 2019, and limited action in the cities to counter air pollution,
the Supreme Court bench again intervened to demand the installation of smog towers and allocated
INR 36 crores (~USD 5.2 million) for the replication of the Xi’an’s smog tower design in Delhi. In
August 2020, a memorandum of understanding was signed by the Indian Institute of Technology
(Bombay) to design and construct the system. Wasting the judicial power by implementing band aid
measures is not only unscientific, but also a waste of limited financial and technical resources. We
cannot vacuum our way to “clean air”.

5. Conclusions
    The city clean air action plans provide proof that there is enough technical know-how on how
much air pollution there is, the key sectors that need attention, the institutional requirements to
implement long-term strategies, and the ways in which they can be addressed [40,41]. These action
plans need institutional and financial support. At the institutional level, there are three tasks that
need immediate attention, where the judiciary can help to move the strategies forward: (1) Personnel
and Capacity— CPCB and the state pollution control boards are too understaffed to perform auditory
Atmosphere 2020, 11, 922                                                                                            9 of 11

and scientific operations. (2) Monitoring infrastructure—as of June 2020, there are 230 continuous
monitoring stations operated and maintained by CPCB in 124 (of 715) districts. More than half of these
districts have only one station and 70 monitors are in the vicinity of the NCR, which demonstrates
the bias in measuring and managing air pollution outside the big cities like Delhi. To spatially and
temporally represent the air pollution problem, India requires at least 4000 continuous air quality
monitoring systems (2800 in the urban areas and 1200 in the rural areas). (3) Information support—air
quality management requires information on emission loads, source contributions, costs and benefits of
interventions, and a way to prioritize actions. The funds allocated by the Supreme Court for temporary
interventions like testing smog towers are most useful for implementing these permanent solutions.

Supplementary Materials: The following are available online at http://www.mdpi.com/2073-4433/11/9/922/s1,
Table S1: Summary of air quality in 124 cities in India for the periods before and during the 4 COVID-19 lockdowns.
Author Contributions: Conceptualization, writing, and editing—S.G. and P.J.; Methodology, resources,
and visualization—S.G. All authors have read and agreed to the published version of the manuscript.
Funding: This research received no external funding.
Conflicts of Interest: The authors declare no conflict of interest.

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