3D bending simulation and mechanical properties of the OLED bending area
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Open Physics 2020; 18: 397–407 Research Article Liang Ma* and Jinan Gu 3D bending simulation and mechanical properties of the OLED bending area https://doi.org/10.1515/phys-2020-0165 devices are attracting more and more attention [1]. People received November 27, 2019; accepted May 30, 2020 have higher requirements with respect to power consump- Abstract: Due to the poor mechanical properties of traditional tion, volume, softness, and other aspects of display devices. simulation models of the organic light-emitting device (OLED) Display devices originated from cathode ray tubes (CRTs). In bending area, this article puts forward a finite element model a CRT, electron flow bombards the screen, so that R, G, and of 3D bending simulation of the OLED bending area. During B phosphors give out light in proportion, thus producing the model construction, it is necessary to determine the different colors. Since the birth of the CRT technology in viscoelastic and hyperelastic mechanical properties, respec- 1897, CRTs were applied in radar display and electronic tively. In order to accurately obtain the stress changes of oscilloscopes at first, and then they were popularized in TVs material deformation during the hyperelasticity determina- and computers, becoming the most mainstream display tion, a uniaxial tensile test and a shear test were used to terminals in the twentieth century [2]. Although CRTs have obtain data and thus to characterize the hyperelastic proper- strong advantages in terms of cost and image quality, their ties. In order to measure the viscoelasticity, a stress relaxation weight, volume, radiation, and energy consumption limit test was used to draw the stress relaxation curve, so as to their development. The dominant position of CRTs is characterize the viscoelastic properties. Then, the plane or gradually replaced by flat panel displays (FPDs). Compared axisymmetric stress–strain analysis was achieved, and the with the traditional CRTs, FPDs have many advantages, material parameters of the 3D model of the OLED bending such as small size, light weight, and low energy consump- area were obtained. Finally, the 3D model was applied to the tion. In recent years, FPDs have developed rapidly. Liquid 3D bending of the OLED bending area. Combined with the crystal displays (LCDs) and plasma display panels (PDPs) axisymmetric finite element analysis method, the 3D bending are the most representative display devices. A pixel in an simulation finite element model of the OLED bending area LCD panel is composed of three LCD units. Each LCD unit was constructed by dividing the finite element mesh. contains a red filter, green filter, or blue filter. Different Experimental results show that the mechanical properties of colors can be generated by controlling the light in different the proposed model are better than those of traditional OLED units [3]. An LCD is thinner than a CRT, which greatly saves bending simulation models. Meanwhile, the proposed model space and avoids the radiation problem. In the aspect of has stronger application advantages. screen refresh rate, a CRT kinescope adopts light-emitting materials. No matter how high the refresh frequency is, it Keywords: OLED, bending area, 3D bending simulation, will lead to the flicker problem. Direct imaging technology mechanical property for LCDs does not cause flicker, so it is more suitable for human eyes. In addition, an LCD is a form of flat screen, and the display effect is much better than that of a CRT. 1 Introduction However, LCDs also have some disadvantages in terms of resolution, viewing angle, color saturation, brightness, and With the rapid development of information age, the infor- reaction speed [4]. A pixel in a PDP is a plasma tube. The mation display technology has become an important branch plasma gas discharges in the plasma tube, producing of the information industry. As information carriers, display ultraviolet light and exciting the phosphor on the fluor- escent screen. A PDP is a kind of self-luminous display technology without backlight, which overcomes the pro- * Corresponding author: Liang Ma, School of Mechanical blems of visual angle and brightness of LCDs. It is easy to Engineering, Jiangsu University, Zhenjiang 212000, China, e-mail: maliang72@163.com manufacture large-scale screens with excellent performance. Jinan Gu: School of Mechanical Engineering, Jiangsu University, However, PDPs have some problems in terms of service life, Zhenjiang 212000, China power consumption, and cost. Open Access. © 2020 Liang Ma and Jinan Gu, published by De Gruyter. This work is licensed under the Creative Commons Attribution 4.0 Public License.
398 Liang Ma and Jinan Gu Although LCDs, PDPs, and other displays solve the small, and the stress changes little with deformation. problems of CRTs in terms of volume, weight, radiation, The measurement scheme is suitable for traditional and screen refresh rate, they still need to be improved in hyperelastic materials, such as rubber, but it cannot be the aspects of energy consumption, viewing angle, and completely suitable for the OCA material due to the brightness. In recent years, LCDs and PDPs have been measurement accuracy. In order to accurately find the unable to meet the growing demand for display stress changes during the material deformation, it is functionality, especially flexible displays [5]. necessary to adopt appropriate instruments and mea- The display of an organic light-emitting device surement schemes. For example, a uniaxial tensile test (OLED) is thinner (its thickness is less than 500 nm), and a simple shear test are used to obtain data and thus and it has the advantages of self-illumination, short to characterize the hyperelastic properties. When deter- response time, large viewing angle, lifelike picture, high mining the viscoelasticity, we can use the stress definition, and low energy consumption. It is a planar relaxation test to get the stress relaxation curve, so as device and is highly compatible with plastic substrates. to characterize the viscoelastic properties. Thus, the During its preparation, low-temperature technology is plane or axisymmetric stress–strain analysis is carried adopted to achieve a flexible display. Compared with out [9]. other flexible displays, it has prominent advantages, as a result of which it gradually became the first choice of flexible displays. In addition, it is rated as the most 2.1.1 Determination and fitting of hyperelastic material potential FPD lighting technology. However, an OLED parameters display is a composite structure composed of thin-film optical devices, and an optical clear adhesive (OCA) is The uniaxial tensile test and simple shear test were used used to make the bonding of all film layers more firm to determine the hyperelasticity of materials. Dynamic [6,7]. An OCA is a special adhesive used for cementing mechanical analysis (DMA) was applied to the uniaxial transparent optical elements. It is required to have tensile test. A rotational rheometer was applied in the colorless transparency, light transmittance above 90%, simple shear test. good cementing strength, curing at room temperature or The thickness h of the specimens prepared by two medium temperature, and curing shrinkage. In the tests is 1 mm. The measurement method is the same as process of bending deformation, the bending radius of the viscoelastic measurement. The OCA samples are flexible OLED modules is small. Meanwhile, various stacked and pasted, and then the specimens are cut as thin-film devices cannot coordinate the deformation. The per the requirements of the chucking appliance [10]. OCA adhesive material has viscous flow, leading to Table 1 shows the size and instrument models of uniaxial device stripping and permanent damage to the screen tensile specimens. Table 2 shows the specifications and [8]. Therefore, a 3D bending simulation model of the instrument models of simple shear specimens. When OLED bending area was built to research the mechanical DMA is adopted for the tensile test, the tensile rate refers properties. to ASTM D412. When the rotary rheometer is adopted for the simple shear test, the shear strain rate is 0.01 s−1. The original data obtained from the experiment are shown in Tables 1 and 2. After processing the data, we 2 Construction of a finite element can get the stress data and strain data. The specific calculation is shown below. model of 3D bending simulation In the uniaxial tensile test, the formula for proces- of the OLED bending area sing stress σT and strain εT is as follows: l − l0 εT = l 2.1 Parameter measurement and fitting of 0 , (1) the OCA material σT = f bh An OCA is a kind of viscoelastic material. It is necessary where l0 is the original length of the specimen, l is the to measure its viscoelastic and hyperelastic mechanical length of the specimen after stretching, f is the tensile properties separately. In the determination of hypere- load, h is the thickness of the specimen, and b is the lasticity, the elastic modulus of the OCA material is too tensile rate.
3D bending simulation and mechanical properties of OLED bending area 399 Table 1: Specimen size and instrument model of the uniaxial tension test Serial number Instrument type DMA TA RSA-G2 1 Sample shape and size Long strip sample, l = 60 mm, B = 6 mm 2 Testing accuracy 0.02 mN Table 2: Specimen size and instrument model of the simple shearing test Serial number Instrument type Rotational rheometer TA DHR-2 1 Sample shape and size Disc specimen, radius r = 40 mm 2 Testing accuracy 0.01 mN Simple tensile test In the simple shearing test, the formula for proces- Uniaxial fitting results sing stress σS and strain γS is as follows: 0.04 Shear fit results Simple shear experiment rϕ 0.035 γS = h , (2) σS = 2τ 0.03 πr 3 Nominal stress / MPa 0.025 where r is the torque of the parallel plate, φ is the rotational displacement of the parallel plate, r is the 0.02 radius, and τ is the shear strain rate. 0.015 The stress and strain formulas of different strain energy density function models under uniaxial tension 0.01 mode and simple shearing mode are obtained by derivation. The derivation formulas are comparable 0.005 with experimental data, and the hyperelastic parameter 0 fitting can be achieved [1]. 0 1 2 3 4 Through the mathematical software 1Stopt, the Nominal strain / 100% formula of stress–strain constitutive relation can be derived. Combined with the experimental data, the Figure 1: Fitting results. fitting results under different strain energy density functions are obtained [11]. After the comparison of the an incompressible material, rather than a completely fitting quality and the judgment of simulation conver- incompressible material in theoretical sense [13]. gence, the reduced polynomial model with N = 3 order is adopted. The fitting results are shown in Figure 1. We can see that the simple shear test data are 2.1.2 Determination and fitting of viscoelastic material basically consistent with the simple shear fitting result. parameters There is a slight difference between the data of the uniaxial tensile test and the uniaxial tensile fitting results, DMA is applied to the viscoelastic stress relaxation test. but they are consistent in the overall trend. On the whole, During the test, the specimens are prepared first. The the fitting effect is very good. After the fitting, relevant thickness of specimens in the DMA test should not be less parameters of the strain energy density function are than 1 mm, while the thickness of the OCA specimen should obtained. The fitting parameters are shown in Table 3 [12]. be less than 0.05 mm. Therefore, it is necessary that the OCA To be clear, the OCA material is an incompressible sample should be cemented, so that the thickness can reach material. Poisson’s ratio v is 0.5. At this time, parameter D1 1 mm. Then, we cut the shape of specimens according to the should be zero. In Abaqus, for materials whose Poisson’s requirements of fixtures and then we can obtain the ratio v is greater than 0.475, Poisson’s ratio v is considered specimens for the experiments. The specification and to be 0.475. That is to say, the material is approximated as instrument model are shown in Table 4.
400 Liang Ma and Jinan Gu Table 3: Fitting parameters of the hyperelastic Yeoh model Normalized experimental data 0.8 Name Fitting parameters Fitting result C10 C20 C30 D1 D2 D3 0.7 Normalized relaxation modulus of elasticity Numerical 0.01061 −0.00012 1.7318 4.79455 0 0 0.6 value × 10−6 0.5 Then, the simple shearing experiment is carried out. 0.4 A 5% instantaneous shear deformation is given to the specimen. It is unchanged, and the change of stress is 0.3 recorded. The data are normalized using equation (3), 0.2 and then the data are input into Abaqus for fitting. The result is shown in Figure 2 [14]. 0.1 N g (t ) = 1 − ∑ gi(1 − e−t /τ ), i (3) 0 0 50 100 150 200 i=1 Time /s where g(t) is the relaxed modulus of elasticity after Figure 2: Fitting results. normalization, t is the relaxation time, N is the number of terms of the Prony series, gi and τi are the parameters in the model, e is the shear threshold, and i is a constant. Table 5: Prony parameters based on viscoelastic fitting For the viscoelastic fitting process of the material, it is only necessary to nondimensionalize the experimental data i 1 2 3 4 5 of stress relaxation in Abaqus, and thus to achieve the plane gi 0.5902 0.1461 0.1115 0.0643 0.0352 or axisymmetric stress–strain analysis. After input, Prony τi 0.0188 0.2084 1.8675 19.167 233.07 parameters gi and τi can be obtained by fitting. Finally, the viscoelastic properties are given to the materials. It can be seen that the fitting curve basically wiring at the end of the bending area is used to transmit coincides with the experimental data curve after the and control the electric signal of the light-emitting diodes normalization. The fitting quality is very good. After in the OLED display area. There are huge amounts of metal fitting, Prony parameters gi and τi are obtained (Table 5). wires deposited in the organic photoresist [15]. The structure of the bending area is shown in Figure 3. According to the structural characteristics of the OLED bending area, OCA material parameters and 2.2 Construction of the 3D model of the membrane material parameters are obtained. The OCA OLED bending area material parameters are shown in Figure 4. The parameters of membrane materials are shown in 2.2.1 Material parameters Table 6. The structure of the OLED bending area is mainly 2.2.2 Construction of the 3D model composed of an organic photoresist, metal wiring, and a polyimide (PI) substrate. The metal wiring at the end of the In order to simplify the OLED bending area, meso- structure is deposited in the organic photoresist. The metal structure information is introduced to characterize the Table 4: Specimen size and instrument model Serial number Instrument type DMA TA RSA-G2 1 Sample shape and size Long strip sample, l = 50 mm, B = 5 mm 2 Testing accuracy 0.01 mN
3D bending simulation and mechanical properties of OLED bending area 401 Table 6: Parameters of membrane materials Back panel material Modulus of Poisson’s ratio elasticity (GPa) Protective cover 5.6 0.29 plate Touch layer 4.076 0.31 Polarizer 3.769 0.33 Display layer 49 0.30 Substrate 9.1 0.33 Backplane 4.2 0.32 Figure 3: Structure of the OLED bending area. Protective cover plate-60 µm OCA-25 µm Figure 5: 3D model of the bending area. Touch layer-50 µm OCA-25 µm Table 7: Geometric parameters Polarizer-47 µm Serial number Material layer Thickness (µm) OCA-20 µm 1 Organic photoresist 4.5 Display layer-10 µm 2 Metal alignment 0.73 Substrate-15 µm 3 Substrate material 1.5 OCA-25 µm 4 PI substrate 15 Backplane-75 µm For the 3D model of the bending area, the geometric parameters of relevant metal lines and material layers Figure 4: OCA rubber parameters. are shown in Table 7. properties of the bending area. The micromechanics of materials are based on the relationship between the macromechanical properties of materials and the micro- 2.3 Construction of the finite element structure. Therefore, the macroproperties can be model of 3D bending simulation of the achieved by optimizing the design of the microstructure. OLED bending area The structure region at the end of the OLED has obvious periodic characteristics [16]. According to the character- 2.3.1 3D bending for the OLED bending area ization of the microstructure, the microstructure of the end structure of the OLED can be composed of an The 3D model of the OLED bending area is combined organic photoresist, single metal wire, substrate mate- with the axisymmetric principle, and the OLED bending rial, and PI substrate. Thus, the 3D model of the bending area is bent in the 3D mode, so that the lower part of the area is built as shown in Figure 5. screen is able to fit with the middle frame. Thus, the
402 Liang Ma and Jinan Gu 150 screen Reference Rigid point body Figure 6: Bending structure and size. screen rotation is achieved. The middle frame can be regarded as a rigid body. In order to form a circular arc at the bending part and reduce the structure stress, the distance between the reference point and the symmetry axis π is set as 4 R mm . When R is 5 mm, the distance is 7.85 mm. The structure and size are shown in Figure 6 [17]. Figure 8: 3D bending simulation model of the OLED bending area. In the first second, the rigid body rotates antic- lockwise around the reference point, at a speed of 1.57 rad/s. At the same time, the rigid body moves to the After bending, the 3D bending simulation model of the π OLED bending area is built as shown in Figure 8. left at a speed of 4 − 1 R mm. The shape after bending is shown in Figure 7. After that, it is placed for 300 s to simulate the actual use. 2.3.2 Grid partition based on axisymmetric finite When the bending radius R = 5 mm, the boundary element analysis condition is that in the first second, the rigid body rotates anticlockwise around the reference point at a According to the 3D bending simulation model of speed of 1.57 rad/s, and then it moves to the left at a the OLED bending area, the finite element model of speed of 2.85 mm/s. Finally, it is placed for 300 s. the three-dimensional bending process is built. First, the axisymmetric finite element analysis method is used to generate the finite element meshes. After bending, the difference between the internal metal wiring width in the OLED bending area and the overall size is large. It is more difficult to generate finite element meshes [18]. It is easy to ignore some characteristics of the metal wiring screen Rigid body structure by using the whole grid division method, influencing the analysis of different metal wiring structures negatively. It is not able to reflect the structural differences of different metal wires. Combined with the principle of axisymmetric finite element R5 analysis, the implicit dynamic viscoelastic analysis method was adopted for the grid division. In order to be consistent with the actual stress situation, the plane Reference point strain grids are adopted. During the mesh generation, the network is quadrilateral, which is convenient for convergence and calculation. The grid size is 0.025 mm. All the membrane materials and OCA materials are divided into three layers. The grid type includes the plane strain unit, hybrid unit, and CPE8RH reduced integration unit. A HyperMesh platform with powerful finite element Figure 7: Shape after bending. preprocessing ability is used for the OLED bending area.
3D bending simulation and mechanical properties of OLED bending area 403 A hexahedron mesh method is used to divide the metal wires and other areas. This can effectively reduce the number of meshes. On this basis, progressive grid division is adopted to ensure the accuracy of the calculated structure and thus to reduce the calculation time. All units in the model are linear hexahedron elements with complete integration [19]. Generally, the accuracy of grid division directly influ- ences the accuracy of the result. The finer the mesh division is, the more accurate the result is. When the grid is too dense, the computer overhead will increase and the computing time will also increase. For the explicit dynamics, the consumption Figure 10: Finite element meshes after the detailed division. of computer memory and computing time are directly proportional to the number of grid units. The computing The details of the division of finite element meshes after cost increases with the improvement of grid subdivision, so the OLED bending are shown in Figure 11. that we can directly predict the cost change caused by grid subdivision. For the implicit dynamics, the computing cost is roughly proportional to the square of the number of freedom 2.3.3 Finite element modeling degrees. The consumption of memory and computing time will have an exponential relationship with the number of grid Refined finite element meshes are used to build the units. It is difficult to predict the cost. The change is obvious. three-dimensional bending simulation finite element On the basis of accuracy, a reasonable grid density can model of the OLED bending area. During the finite greatly optimize the computing cost. For the structure of the OLED bending area, on the premise of reflecting the structural features of the metal wire, we must refine the grid as much as possible, so that the grid size can ensure the computing accuracy without consuming too much com- puting resource [20]. Due to the ratio of the length and thickness of the OLED bending area after bending, the number of metal wiring meshes is still huge on the basis of accuracy, consuming too much computer resource. In order to improve the accuracy of calculation and analysis, a sub- model is used to divide the structure of the OLED bending area after bending. There are 26 × 30 divided finite element grids, as shown in Figure 9. On this basis, the finite element meshes are divided in detail. The specific results are shown in Figure 10. Figure 11: Details of the finite element mesh after the detailed Figure 9: Finite element mesh. division: (a) details of finite element mesh and (b) enlarged details.
404 Liang Ma and Jinan Gu element simulation, the setting of boundary condition load directly influences the success of simulation. This is also an extremely important part of finite element simulation. In the finite element simulation, there are two ways to Global boundary conditions realize the periodic boundary: (1) coupling corre- sponding surface nodes. This method has higher requirements for serial number of nodes, but it can reduce constraints and improve calculation accuracy. (2) A penalty function is introduced. The implementation of this method is simple, but it is easy to cause a numerical difference. Therefore, the periodic boundary constraints can be achieved by combining these two methods. The special boundary constraint needs to divide the whole z model into two independent models: a global model and a sub-model. The global model includes a geometric x constraint, displacement constraint, and boundary con- y straint. The sub-model is a part of the whole model, so we cannot analyze the global features of the model, such as cracks. In the global model, the displacement corresponding to the sub-model is the boundary condi- load tion of the sub-model. Therefore, the grid of the global model is relatively coarse. If the global model corre- Figure 12: Global model. sponds to the sub-model, the calculation results will be more accurate [21]. bending speed is expanded n times, the calculation time will The basic implementation steps of special boundary 1 be shortened to n of the original time. In order to ensure that constraints in the finite element analysis include the following: the energy distribution in the simulation process is (1) global model analysis: the global model is divided consistent with the actual situation, the simulation speed with coarse meshes without considering the local should be stable. Therefore, the bending speed is set as structure details, and then the global structure is 3,000 mm/s, the optimal bending radius is 2 mm, and the analyzed to calculate the displacement at a specific time to complete the simulation is 2.444 s. Then, the location (near the boundary of the sub-model). amplitude curve of finite element analysis is obtained. The (2) establishment of the sub-model: according to the specific process is shown in Figure 14. analysis target and the actual structure, the sub- model of a local fine mesh is built. (3) boundary condition interpolation value: the displa- Sub boundary conditions / loads cement boundary of the global model obtained in the first step is taken as the boundary condition. Then, it is automatically loaded to the corresponding position in the sub-model by the linear interpolation method (the displacement interpolation result de- termines the computing accuracy of the sub-model). (4) result analysis of the sub-model: the original boundary and load in the region of sub-models are unchanged, and then the finite element analysis is performed on sub-models. The global model is shown z in Figure 12, and the sub-model is shown in Figure 13. x In the setting of boundary conditions, the efficiency of y calculation can be improved by increasing the bending speed under the condition of a constant time step. If the Figure 13: Sub-model.
3D bending simulation and mechanical properties of OLED bending area 405 Table 8: Parameters of each material layer in the finite element model Open. DXF format file Material layer Young’s Poisson’s ratio modulus (Mpa) PI substrate 9,200 0.35 Organic photoresist 3,400 0.35 Read. DXF format file Metal alignment 80,000 0.35 Inorganic substrate 1,10,000 0.17 According to the amplitude curve of finite element analysis, HyperMesh software is used to build the finite Calculate interpolation Enter sample interval element model of three-dimensional bending simulation point value of the OLED bending area. The specific model is shown in Figure 15. Enter bending speed Calculating displacement 3 Research on mechanical properties array 3.1 Experimental process The mechanical properties in the bending process of the Get the amplitude curve of OLED bending area were researched using the 3D Input channel spacing finite element analysis compress stretching Figure 14: Specific process of obtaining the amplitude curve of finite element analysis. Protective cover plate 60 µm OCA1 25 µm Touch layer 50 µm OCA2 25 µm Polarizer 47 µm OCA3 20 µm Display layer 10 µm Substrate 15 µm OCA4 25 µm Backplane-75 µm -0.02 -0.015 -0.01 -0.005 0 0.005 0.01 0.015 0.02 Nominal strain / 100% Periodic boundary condition algorithm Special boundary constraints Bending mechanical response Figure 15: Finite element model of 3D bending simulation of the Figure 16: Experimental results of mechanical properties of OLED bending area. traditional models.
406 Liang Ma and Jinan Gu compress stretching Protective cover plate 60 µm OCA1 25 µm Touch layer 50 µm OCA2 25 µm Polarizer 47 µm OCA3 20 µm Display layer 10 µm Substrate 15 µm OCA4 25 µm Backplane-75 µm -0.02 -0.015 -0.01 -0.005 0 0.005 0.01 0.015 0.02 Nominal strain / 100% Periodic boundary condition algorithm Special boundary constraints Bending mechanical response Figure 17: Experimental results of mechanical properties of the proposed model. bending simulation finite element model of the OLED mechanical properties of three traditional OLED bending bending area [22–25]. First, the material parameters of simulation models are shown in Figure 16. each layer in the finite element model were calculated. The experimental results of the mechanical properties of The specific results are shown in Table 8. the finite element model of three-dimensional bending In order to ensure the fairness and effectiveness of simulation of the OLED bending area are shown in Figure 17. the experimental results, three traditional bending According to the verification results of mechanical simulation models such as the model based on a periodic properties, the performance of strain distribution of the boundary condition algorithm, the model based on finite element model of three-dimensional bending special boundary constraints, and the model based on simulation of the OLED bending area is better than bending mechanical response were used to compare the that of the traditional model, so that the effectiveness of finite element model designed in this article. The the proposed model can be proved. mechanical properties of the proposed model were judged using the strain distribution [26,27]. The more tortuous the strain distribution curve is, the stronger the strain distribution performance is. 4 Conclusions Due to the poor mechanical properties obtained in the traditional simulation models of the OLED bending area, 3.2 Research results a finite element model for three-dimensional bending simulation of the OLED bending area is proposed. This In this study, the mechanical properties of the bending model effectively improves the mechanical properties, so region were analyzed by observing the motion states at it has great significance for the research on the bending different positions. The experimental results of the properties of OLED screens.
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